GameOverCast discuss their unrequited love with Portal 2
I already asked NickWorks about it and he promptly never responded.
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It's all coming back to me now...
I offered to buy his site too. Which he also never responded.
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The similarity to Valve's official Portal 2 site URL counts a little bit as well 
http://www.soundcloud.com/jomonay
"Anything that you do, just be THE best at it" - Kanye West
Speaking of selling domains, I'm shocked they never offered to buy it.
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"Think with portals" would be used in the future tense (eg "I will think with portals"), while "Thinking with portals" would be used more in the present tense (eg. "I am thinking with portals"). Valve's choice makes sense seeing as its primary purpose was to persuade people to pre-order the game, but now it's released, it can be seen as a command (eg "Think with portals now"), which could encourage pepole to buy it.
Over-analysis complete.
http://www.soundcloud.com/jomonay
"Anything that you do, just be THE best at it" - Kanye West
Valve's choice was "fuck, this asshole got the domain we should have before we released that trailer, this one is close enough".
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What can I say, you're forward thinking if nothing else
http://www.soundcloud.com/jomonay
"Anything that you do, just be THE best at it" - Kanye West
FTFY.